The "./rho0-to10800-topo500.tbl" "./rho1-to10800-topo500.tbl" files contain spherical harmonic coefficients of the zero- and first-order polynomial density coefficients of the lunar crust as represented by Eq. (4) of Bucha (2025). The coefficients were derived from the 3D linear crustal density model of Goossens et al. (2020) using the LIN_L250-650_TC40_rho.grd LIN_L250-650_TC40_grad.grd grids. First, the grids of Goossens et al. (2020) was transformed into the representation required by Eq. (4) of Bucha (2025) using Eq. (45) of Bucha (2025). The "rS" term in Eq. (45) of Bucha (2025) was obtained by the surface spherical harmonic synthesis of "../topo/Moon_LDEM128_shape_pa_11519.tbl" up to degree 500. Finally, the grids of "rho0" and "rho1" were harmonically analyzed up to degree 10800 to mitigate aliasing. The "./rho0-to10800-topo5400.tbl" "./rho1-to10800-topo5400.tbl" files are similar to "./rho0-to10800-topo500.tbl" "./rho1-to10800-topo500.tbl" with the difference being in the degree, up to which "rS" was expanded. In this case, "rS" was expanded to degree 5400. The file structure follows the CHarm's "tbl" file format (see "https://www.charmlib.org"). The coefficients are "4pi"-fully-normalized and exclude the Condon--Shortley phase factor. NOTE 1: The coefficients depend on the truncation degree of the lunar shape "rS" and they must always be used with the same topography expanded up to the same truncation degree. NOTE 2: To get the density, both sets of coefficients ("rho0" and "rho1") must always be used together. Using only "rho0" will *not* yield laterally variable density of the lunar crust. See Bucha (2025) for details. REFERENCES: Bucha, B. 2025. Spectral gravity forward modelling of 3D variable densities using an arbitrary integration radius with application to lunar topographic masses. Journal of Geodesy, 99:31 https://doi.org/10.1007/s00190-025-01951-9 Goossens S., Sabaka T. J., Wieczorek M. A., Neumann G. A., Mazarico E., Lemoine F. G., Nicholas J. B., Smith D. E., Zuber M. T. (2020) High-resolution gravity field models from GRAIL data and implications for models of the density structure of the Moon's crust. Journal of Geophysical Research: Planets 125:e2019JE006086, https://doi.org/10.1029/2019JE006086$